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Synthesis of nanoporous aluminosilicate materials and their application as highly selective heterogeneous catalysts for the synthesis of β-amino alcohols

Robinson, M. C. W., Davies, A. M., Mabbet, I., Davies, T.E., Apperley, D. C., Taylor, Stuart Hamilton and Graham, A. E. 2010. Synthesis of nanoporous aluminosilicate materials and their application as highly selective heterogeneous catalysts for the synthesis of β-amino alcohols. Journal of Molecular Catalysis A: Chemical 329 (1-2) , pp. 57-63. 10.1016/j.molcata.2010.06.018

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Abstract

The ability of nanoporous aluminosilicate materials, synthesized using an evaporation-induced self-assembly (EISA) approach, to function as catalysts for the formation of β-amino alcohols from aromatic amines and epoxides was assessed. Materials containing high aluminium loadings displayed catalytic activity, giving the desired β-amino alcohols in high yield and with high selectivity for the Markovnikov addition product. These materials exhibited nanoporous pores, typically 1.34-1.49 nm, with a narrow pore size distribution and the expected large surface areas. © 2010 Elsevier B.V.

Item Type: Article
Status: Published
Schools: Chemistry
Cardiff Catalysis Institute (CCI)
Neuroscience and Mental Health Research Institute (NMHRI)
Subjects: Q Science > QD Chemistry
Uncontrolled Keywords: Addition products; Aluminosilicate materials; Amino alcohols; Aromatic amines; Catalytic activity; Evaporation-induced self-assembly; Heterogeneous catalyst; High selectivity; High yield; Large surface area; Lewis acid catalysts; Nano-porous; Narrow pores, Acids; Alcohols; Aluminosilicates; Amination; Catalysts; Evaporation; Pore size; Self assembly, Amines
Additional Information: cited By (since 1996) 3
Publisher: Elsevier BV
ISSN: 13811169
Last Modified: 04 Jun 2017 02:10
URI: http://orca.cf.ac.uk/id/eprint/10233

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