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Involvement of surface-bound radicals in the oxidation of toluene using supported Au-Pd nanoparticles

Saiman, Mohd Izham, Brett, Gemma Louise, Tiruvalam, Ramchandra, Forde, Michael M., Sharples, Katherine Mary, Thetford, Adam, Jenkins, Robert Leyshon, Dimitratos, Nikolaos, Lopez-Sanchez, Jose Antonio, Murphy, Damien Martin, Bethell, Donald, Willock, David James, Taylor, Stuart Hamilton, Knight, David Wiliam, Kiely, Christopher John and Hutchings, Graham John 2012. Involvement of surface-bound radicals in the oxidation of toluene using supported Au-Pd nanoparticles. Angewandte Chemie. International Edition 51 (24) , pp. 5981-5985. 10.1002/anie.201201059

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Abstract

Au-Pd nanoparticles having a mean particle size of 3–4 nm and supported on titania (see figure; scale bar 2 nm) exhibit high activity in the selective oxidation of aromatic hydrocarbons using tert-butyl hydroperoxide as an oxidant. The supported nanoparticles stabilize surface-bound radicals.

Item Type: Article
Date Type: Publication
Status: Published
Schools: Cardiff Catalysis Institute (CCI)
Chemistry
Subjects: Q Science > QD Chemistry
Uncontrolled Keywords: alloys; gold; heterogeneous catalysis; nanoparticles; palladium
Publisher: Wiley-Blackwell
ISSN: 1433-7851
Funders: Dow Chemical Company
Last Modified: 06 Sep 2019 23:31
URI: http://orca.cf.ac.uk/id/eprint/23662

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