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Kinetics of iminium ion catalysis

Evans, Gareth James, Gibbs, Timothy John, Jenkins, Robert Leyshon, Coles, Simon J., Hursthouse, Michale B., Platts, James Alexis and Tomkinson, Nicholas Charles Oliver 2008. Kinetics of iminium ion catalysis. Angewandte Chemie. International Edition 47 (15) , pp. 2820-2823. 10.1002/anie.200705539

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Abstract

Identifying the bottleneck: Kinetic and computational data for the key steps of the iminium ion catalyzed Diels–Alder reaction show that the cycloaddition (step II in scheme) is the rate-determining step of the catalytic cycle and provide a rationale for developing more-active catalyst architectures.

Item Type: Article
Date Type: Publication
Status: Published
Schools: Chemistry
Uncontrolled Keywords: cycloaddition ; Density functional calculations ; Iminium ions ; Kinetics ; Organocatalysis
Publisher: Wiley
ISSN: 1433-7851
Last Modified: 18 Oct 2017 12:35
URI: http://orca.cf.ac.uk/id/eprint/5934

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