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Thiocyanate complexes of uranium in multiple oxidation states: a combined structural, magnetic, spectroscopic, spectroelectrochemical and theoretical study

Hashem, Emtithal, Platts, James Alexis, Hartl, František, Lorusso, Giulia, Evangelisti, Marco, Schulzke, Carola and Baker, Robert J. 2014. Thiocyanate complexes of uranium in multiple oxidation states: a combined structural, magnetic, spectroscopic, spectroelectrochemical and theoretical study. Inorganic Chemistry 53 (16) , pp. 8624-8637. 10.1021/ic501236j

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Abstract

Uranium thiocyanate complexes in different oxidation states have been studied by SQUID magnetometry, photoluminescence spectroscopy, and spectroelectrochemistry. The magnetic properties of [U(NCS)8]4− have been studied with respect to the geometry around the uranium ion. The thiocyanate ligands in this complex have been found to undergo unusual anodic reactivity.

Item Type: Article
Date Type: Publication
Status: Published
Schools: Chemistry
Advanced Research Computing @ Cardiff (ARCCA)
Subjects: Q Science > QD Chemistry
Uncontrolled Keywords: Uranium; magnetic properties; photoluminescence; DFT.
Publisher: American Chemical Society
ISSN: 0020-1669
Date of Acceptance: 29 July 2014
Last Modified: 12 Aug 2019 14:27
URI: http://orca.cf.ac.uk/id/eprint/62517

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