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Heterodyne spectral interferometry for multidimensional nonlinear spectroscopy of individual quantum systems

Langbein, Wolfgang Werner and Patton, Brian 2006. Heterodyne spectral interferometry for multidimensional nonlinear spectroscopy of individual quantum systems. Optics Letters 31 (8) , pp. 1151-1153. 10.1364/OL.31.001151

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Abstract

A novel implementation of transient nonlinear spectroscopy is presented that allows the study of the transient nonlinear polarization emitted from individual electronic transitions. Both the amplitude and the phase of the polarization are retrieved, permitting the implementation of multidimensional spectroscopy in the excitation pulse delays. The technique is shown to detect mutual coherent coupling in a group of individual, localized excitonic transitions.

Item Type: Article
Date Type: Publication
Status: Published
Schools: Physics and Astronomy
Subjects: Q Science > QC Physics
Publisher: Optical Society of America
ISSN: 0146-9592
Last Modified: 04 Jun 2017 08:00
URI: http://orca.cf.ac.uk/id/eprint/71369

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