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Palladium-tin catalysts for the direct synthesis of H2O2 with high selectivity

Freakley, Simon J., He, Qian, Harrhy, J. H., Lu, L., Crole, D. A., Morgan, David John, Ntainjua, E. N., Edwards, Jennifer Kelly, Carley, Albert Frederick, Borisevich, A. Y., Kiely, Christopher J. and Hutchings, Graham John 2016. Palladium-tin catalysts for the direct synthesis of H2O2 with high selectivity. Science 351 (6276) , pp. 965-968. 10.1126/science.aad5705

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Abstract

Hydrogen peroxide is synthesized industrially without direct contact of hydrogen and oxygen in order to achieve high concentrations. For many applications, only dilute aqueous solutions are needed. Freakley et al. report an improvement in the direct synthesis of hydrogen peroxide over using palladium-tin alloys. This catalyst still achieves selectivities of >95%, like palladium-gold alloys, but is cheaper and can suppress reactions that decompose the product.

Item Type: Article
Date Type: Publication
Status: Published
Schools: Cardiff Catalysis Institute (CCI)
Chemistry
Subjects: Q Science > QD Chemistry
Publisher: American Association for the Advancement of Science
ISSN: 0036-8075
Last Modified: 25 May 2018 19:36
URI: http://orca.cf.ac.uk/id/eprint/87603

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